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Kinetics of microwave-enhanced oxidation of phenol by hydrogen peroxide

Deming ZHAO, Jie CHENG, Michael R. HOFFMANN

《环境科学与工程前沿（英文）》 2011年 第5卷 第1期   页码 57-64 doi: 10.1007/s11783-010-0251-9

摘要： Aqueous solutions of phenol were oxidized by hydrogen peroxide assisted by microwave (MW) irradiation. A simple kinetic model for the overall degradation of phenol in the presence of excess H O is proposed in which the degradation rate of phenol is expressed as a linear function of the concentrations of phenol and H O . A detailed parametric study showed that the degradation rate of phenol increased with increasing [H O ] until saturation was observed. Phenol degradation followed apparent zero-order kinetics under MW radiation or H O oxidation. However, after 90 min of irradiation, the observed kinetics shifted to pseudo first order. The overall reaction rates were significantly enhanced in the combined MW/H O system, mainly because microwave could accelerate H O to generate hydroxyl radical ( OH) and other reactive oxygen intermediates. The observed synergetic effects of the MW/H O process resulted in an increased in the net reaction rate by a factor of 5.75. When hydrogen peroxide is present in a large stoichiometric excess, the time required to achieve complete mineralization is reduced significantly.

关键词： microwave (MW) irradiation     hydrogen peroxide     phenol     synergetic effects     kinetic model    

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Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1632-1

摘要：

● NH3 in biogas had a slight inhibitory effect on dry reforming.

关键词： Biogas     Dry reforming     Sulfur poisoning     Ammonia     Synergetic effect     Hydrogen    

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重大建设工程技术创新网络协同要素与协同机制分析

王孟钧,刘慧,张镇森,陆洋

《中国工程科学》 2012年 第14卷 第12期   页码 106-112

摘要：

通过文献研究、现场调研以及访谈等方式，认为工程需求、组织、资源、制度是重大建设工程技术创新网络的4个协同要素，构建由合作机制、利益机制、激励机制和评价机制组成的协同机制模型，并论证通过协同机制的有效运行，能够提升重大建设工程技术创新能力和效率。 本研究为建设工程技术创新网络理论研究的组成部分，对建设工程技术创新实践活动以及制定行业技术创新政策具有一定的理论参考价值。

关键词： 重大建设工程     技术创新网络     协同要素     协同机制    

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Synergetic Management Theory for Coal-Based Energy Engineering and the Engineering Practice of Shenhua

Wen Ling

《工程管理前沿（英文）》 2016年 第3卷 第1期   页码 1-8 doi: 10.15302/J-FEM-2016005

摘要： To deal with problems in synergetic development of coal-based energy engineering, this paper, guided by the philosophy of engineering, proposes the synergetic management philosophy of “factors coordination, systems synergy, dynamic optimization and three-dimension planning.” The paper also establishes the synergetic management system characterized by systems factor synergy, resource-environment synergy and systems boundary extension and supported by the “two-wheel driven” management innovation and technological innovation. In addition, the paper presents a multi-objective dynamic optimization model for energy engineering, designed based on Shenhua’s own engineering practice, to analyze Pareto optimal solution in three scenarios: best resource allocation, minimal environmental impact and maximal value creation. This provides important reference to synergetic development strategies and decision-making in engineering management.

关键词： coal-based energy     engineering synergetic management     two-wheel driven innovation     Shenhua engineering    

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藏北高原草地生态治理与畜牧业协同发展模式研究

干珠扎布,胡国铮,高清竹,江村旺扎,旦久罗布,参木友,巴桑旺堆,杨富裕,魏学红,杨永平

《中国工程科学》 2019年 第21卷 第5期   页码 93-98 doi: 10.15302/J-SSCAE-2019.05.013

摘要：

藏北高原是我国重要的生态安全屏障和高原特色畜牧业基地，而高寒草地退化严重制约着其生态和生产功能，给生态保护和畜牧业发展带来了挑战。本文在深入分析藏北高原生态治理与畜牧业发展状况的基础上，探讨了藏北高寒草地生态与生产功能的主要影响因素，提出了藏北高原草地生态治理与畜牧业协同发展的模式体系。研究表明，通过草地生态恢复、优化放牧管理方式、人工牧草种植、低海拔农区种草高海拔牧区养畜的“低草高牧”模式、冬季半舍饲养殖等一系列措施，能够推进高寒草地生态功能提升、促进草地畜牧业转型升级，实现“保护中发展”与“发展中保护”。相关研究将为治边稳藏、保障国家生态安全、增加牧民收入提供战略引导和科技支撑。

关键词： 藏北高原     生态修复     草地畜牧业     协同发展    

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Temporal variation of PM-associated health effects in Shijiazhuang, Hebei

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1376-0

摘要：

•Annual mean PM2.5 in Shijiazhuang were 87, 95, and 82 µg/m3 in 2015–2017.

关键词： PM2.5     Health effects     Integrated exposure-response model     Shijiazhuang    

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Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1506-3

摘要：

• The early corrosion process in the cast iron pipes was investigated.

关键词： Cast iron pipe corrosion     Drinking water distribution systems     Chlorine disinfection     Iron-oxidizing bacteria     Coupling effects    

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Investigation of effects of Cocamide Diethanolamide chemical on physical and rheological properties of

《结构与土木工程前沿（英文）》 2022年 第16卷 第1期   页码 99-116 doi: 10.1007/s11709-021-0799-4

摘要： In this study, bituminous binder was modified with Cocamide Diethanolamide chemical, a non-ionic surfactant, and the physical and rheological properties of modified binders were investigated. In addition, Cocamide Diethanolamide has been used for the first time to modify bituminous binder, and this situation makes the study distinctive. Bituminous binder was modified more than once with the chemical by changing modification parameters and using certain additive ratios (1%, 3%, and 5%). The effects of different modification parameters and chemical additive on modified samples were investigated with conventional bitumen tests (softening point, penetration, ductility) and Superpave tests (rotational viscometer, rolling thin film oven test, pressure aging vessel, dynamic shear rheometer, bending beam rheometer). In addition, the structural characteristics of the reference binder and modified samples were examined by X-ray diffraction, Fourier Transform Infrared Spectroscopy, scanning electron microscopy, and energy dispersive X-ray spectroscopy. The examinations showed that Cocamide Diethanolamide softens bituminous binder and lowers processing temperatures. In addition, compared to reference binder, rutting resistances of modified bituminous binders decreased with the increase of additive ratio. However, modification with Cocamide Diethanolamide increased the resistance to fatigue cracks and thermal cracks.

关键词： Cocamide Diethanolamide     bitumen modification     rheology     Superpave tests    

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Protective effects of lignin fractions obtained from grape seeds against bisphenol AF neurotoxicity viaantioxidative effects mediated by the Nrf2 pathway

《化学科学与工程前沿（英文）》 2023年 第17卷 第7期   页码 976-989 doi: 10.1007/s11705-022-2237-0

摘要： Lignin exhibits antioxidative and various other biological properties. However, its neuroprotection capability has rarely been studied. In this study, three types of lignin with different structures were prepared from grape seeds by using different isolation techniques. The antioxidative and neuroprotective effects of the lignin fractions were evaluated with the apoptosis model of murine neuroectodermal (NE-4C) neural stem cells stimulated with bisphenol AF. The results demonstrated that the half maximal inhibitory concentration for scavenging 2,2-diphenyl-1-picrylhydrazyl with water-soluble lignin (L-W, 58.19 μg·mL–1) was lower than those of lignin in the autohydrolyzed residue of grape seeds (84.27 μg·mL–1) and original lignin in grape seeds (99.44 μg·mL–1). BPAF exposure had negative effects on the reactive oxygen species, malondialdehyde content, and superoxide dismutase and glutathione peroxidase activities in NE-4C cells, which can be reversed by using the prepared lignin to reduce oxidative stress. An immunofluorescence assay demonstrated that grape seed lignin induced protective effects on BPAF-injured NE-4C cells via the nuclear factor erythroid 2-related Factor 2 pathway. In addition, correlational analyses showed that lignin (L-W) with lower molecular weights and noncondensed phenolic hydroxyl group content and higher contents of COOH groups effectively prevented cell apoptosis, scavenged reactive oxygen species, and ensured protection from nerve injury. This study demonstrated that grape seed lignin can be used as a neuroprotective agent and serves as a demonstration of active lignin production from grape seed waste.

关键词： grape seed lignin     structure     antioxidant     NE-4C cells     neuroprotection    

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Quorum sensing regulation methods and their effects on biofilm in biological waste treatment systems:

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1495-2

摘要：

• Quorum sensing enhancement and inhibition methods are summarized.

关键词： Quorum sensing     Biological waste treatment     Biofilm formation    

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Seismic effects on reinforcement load and lateral deformation of geosynthetic-reinforced soil walls

《结构与土木工程前沿（英文）》 2021年 第15卷 第4期   页码 1001-1015 doi: 10.1007/s11709-021-0734-8

摘要： Current design methods for the internal stability of geosynthetic-reinforced soil (GRS) walls postulate seismic forces as inertial forces, leading to pseudo-static analyses based on active earth pressure theory, which yields unconservative reinforcement loads required for seismic stability. Most seismic analyses are limited to the determination of maximum reinforcement strength. This study aimed to calculate the distribution of the reinforcement load and connection strength required for each layer of the seismic GRS wall. Using the top-down procedure involves all of the possible failure surfaces for the seismic analyses of the GRS wall and then obtains the reinforcement load distribution for the limit state. The distributions are used to determine the required connection strength and to approximately assess the facing lateral deformation. For sufficient pullout resistance to be provided by each reinforcement, the maximum required tensile resistance is identical to the results based on the Mononobe–Okabe method. However, short reinforcement results in greater tensile resistances in the mid and lower layers as evinced by compound failure frequently occurring in GRS walls during an earthquake. Parametric studies involving backfill friction angle, reinforcement length, vertical seismic acceleration, and secondary reinforcement are conducted to investigate seismic impacts on the stability and lateral deformation of GRS walls.

关键词： geosynthetics     reinforced soil     retaining walls     seismic performance    

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Effects of manufactured nanomaterials on algae: Implications and applications

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1554-3

摘要：

● Summary of positive and negative effects of MNMs on algae.

关键词： Manufactured nanomaterials     Algae     Mechanisms     Effects     Implications     Applications    

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Modeling radiative effects of haze on summer-time convective precipitation over North China: a case study

Xuying WANG, Bin ZHANG

《环境科学与工程前沿（英文）》 2016年 第10卷 第4期 doi: 10.1007/s11783-016-0840-3

摘要： We modeled the impact of haze radiative effects on precipitation in North China. Shortwave heating induced by haze radiative effects would reduce heavy rainfalls. Convection was the key factor that whether precipitation was enhanced or suppressed. Precipitation was often suppressed where CAPE, RH and updraft velocities were high. The impact of haze radiative effect on summertime 24-h convective precipitation over North China was investigated using WRF model (version 3.3) through model sensitivity studies between scenarios with and without aerosol radiative effects. The haze radiative effect was represented by incorporating an idealized aerosol optical profile, with AOD values around 1, derived from the aircraft measurement into the WRF shortwave scheme. We found that the shortwave heating induced by aerosol radiative effects would significantly reduce heavy rainfalls, although its effect on the post-frontal localized thunderstorm precipitation was more diverse. To capture the key factors that determine whether precipitation is enhanced or suppressed, model grids with 24-h precipitation difference between the two scenarios exceeding certain threshold (>30 mm or<-30 mm) were separated into two sets. Analyses of key meteorological variables between the enhanced and suppressed regimes suggested that atmospheric convection was the most important factor that determined whether precipitation was enhanced or suppressed during summertime over North China. The convection was stronger over places with precipitation enhancement over 30 mm. Haze weakened the convection over places with precipitation suppression exceeding 30 mm and caused less water vapor to rise to a higher level and thus further suppressed precipitation. The suppression of precipitation was often accompanied with relatively high convective available potential energy (CAPE), relative humidity (RH) and updraft velocities.

关键词： Haze     Aerosol radiative effects     Convective precipitation    

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Interactive effects of high-speed rail on nodal zones in a city: exploratory study on China

Guo LIU, Kunhui YE

《工程管理前沿（英文）》 2019年 第6卷 第3期   页码 327-335 doi: 10.1007/s42524-019-0051-2

摘要： The arrival of the high-speed rail (HSR) era has accelerated the pace of urban development, but its broad socioeconomic impact remains subject to intense debates. This research aims to propose a model for measuring the impact of HSR operation on HSR stations and the surrounding areas, which this research call the HSR-based nodal zone (HNZ). The proposed model is composed of two variables (i.e., transportation situation and vitality) and three subsystems (i.e., economic, societal, and environmental). Data were collected in China through questionnaire survey. Results indicate that the effects of HSR operation on HNZ are multidimensional, transportation vitality has an intermediary role in the effects, and the effects on the physical environment are negative. This study presents an early examination of the impact of HSR operation on the HSR stations and relevant areas and contributes new evidence to academic debates on the contribution of HSR to urban development. Accordingly, urban development policies should be built on the mechanism of HSR in driving the growth of HNZ.

关键词： high-speed rail     nodal zone     interactive effects     sustainable urbanization     China    

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Higher-order mode effects on the seismic performance of tall piers

Zhongguo GUAN, Jianzhong LI, Yan XU, Hao LU

《结构与土木工程前沿（英文）》 2011年 第5卷 第4期   页码 496-502 doi: 10.1007/s11709-011-0131-9

摘要： A comprehensive analysis was conducted to investigate the seismic performance of a typical tall bridge pier through incremental dynamical analysis (IDA). The effect of higher-order modes was studied specifically. The results showed that higher-order modes significantly contributed to the structural seismic response and should not be neglected. Including these modes resulted in an additional hinge midway up the pier. No plastic hinge would occur at this location for conventional bridge piers. Higher-order modes also led to an out-of-phase response between the hinge rotation at the pier bottom and the displacement at the top. This means that the displacement-based seismic design method cannot correctly predict the mechanical state of the critical hinge and therefore is not suitable for use in the seismic design of tall piers. Mistakenly using the displacement-based seismic design method for tall piers may result in a seriously unsafe condition.

关键词： tall bridges     higher-order mode effects     incremental dynamic analysis    

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标题 作者 时间 类型 操作

Kinetics of microwave-enhanced oxidation of phenol by hydrogen peroxide

Deming ZHAO, Jie CHENG, Michael R. HOFFMANN

期刊论文

Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

期刊论文

重大建设工程技术创新网络协同要素与协同机制分析

王孟钧,刘慧,张镇森,陆洋

期刊论文

Synergetic Management Theory for Coal-Based Energy Engineering and the Engineering Practice of Shenhua

Wen Ling

期刊论文

藏北高原草地生态治理与畜牧业协同发展模式研究

干珠扎布,胡国铮,高清竹,江村旺扎,旦久罗布,参木友,巴桑旺堆,杨富裕,魏学红,杨永平

期刊论文

Temporal variation of PM-associated health effects in Shijiazhuang, Hebei

期刊论文

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

期刊论文

Investigation of effects of Cocamide Diethanolamide chemical on physical and rheological properties of

期刊论文

Protective effects of lignin fractions obtained from grape seeds against bisphenol AF neurotoxicity viaantioxidative effects mediated by the Nrf2 pathway

期刊论文

Quorum sensing regulation methods and their effects on biofilm in biological waste treatment systems:

期刊论文

Seismic effects on reinforcement load and lateral deformation of geosynthetic-reinforced soil walls

期刊论文

Effects of manufactured nanomaterials on algae: Implications and applications

期刊论文

Modeling radiative effects of haze on summer-time convective precipitation over North China: a case study

Xuying WANG, Bin ZHANG

期刊论文

Interactive effects of high-speed rail on nodal zones in a city: exploratory study on China

Guo LIU, Kunhui YE

期刊论文

Higher-order mode effects on the seismic performance of tall piers

Zhongguo GUAN, Jianzhong LI, Yan XU, Hao LU

期刊论文